Bottom-up approach to making larger hydrocarbon molecules capable of optical cycling

Krantz, P. et al. A quantum engineer’s guide to superconducting qubits. Appl. Phys. Rev. 6, 021318 (2019).

Article  Google Scholar 

Zwanenburg, F. A. et al. Silicon quantum electronics. Rev. Mod. Phys. 85, 961 (2013).

Article  CAS  Google Scholar 

Kaufman, A. M. & Ni, K.-K. Quantum science with optical tweezer arrays of ultracold atoms and molecules. Nat. Phys. 17, 1324–1333 (2021).

Article  CAS  Google Scholar 

Bruzewicz, C. D., Chiaverini, J., McConnell, R. & Sage, J. M. Trapped-ion quantum computing: progress and challenges. Appl. Phys. Rev. 6, 021314 (2019).

Article  Google Scholar 

Carr, L. D., DeMille, D., Krems, R. V. & Ye, J. Cold and ultracold molecules: science, technology and applications. New J. Phys. 11, 055049 (2009).

Article  Google Scholar 

Albert, V. V., Covey, J. P. & Preskill, J. Robust encoding of a qubit in a molecule. Phys. Rev. X 10, 031050 (2020).

CAS  Google Scholar 

Jain, S. P., Hudson, E. R., Campbell, W. C. & Albert, V. V. Absorption–emission codes for atomic and molecular quantum information platforms. Phys. Rev. Lett. 133, 260601 (2024).

Article  CAS  PubMed  Google Scholar 

Isaev, T. A. & Berger, R. Polyatomic candidates for cooling of molecules with lasers from simple theoretical concepts. Phys. Rev. Lett. 116, 063006 (2016).

Article  PubMed  Google Scholar 

Kozyryev, I., Baum, L., Matsuda, K. & Doyle, J. M. Proposal for laser cooling of complex polyatomic molecules. ChemPhysChem 17, 3641–3648 (2016).

Article  CAS  PubMed  Google Scholar 

Augenbraun, B. L., Doyle, J. M., Zelevinsky, T. & Kozyryev, I. Molecular asymmetry and optical cycling: laser cooling asymmetric top molecules. Phys. Rev. X 10, 031022 (2020).

CAS  Google Scholar 

Dickerson, C. E. et al. Franck–Condon tuning of optical cycling centers by organic functionalization. Phys. Rev. Lett. 126, 123002 (2021).

Article  CAS  PubMed  Google Scholar 

Fitch, N & Tarbutt, M. in Advances in Atomic, Molecular, and Optical Physics Vol. 70 (eds Dimauro, L. F. et al.) 157–262 (Elsevier, 2021).

Vilas, N. B. et al. Magneto-optical trapping and sub-Doppler cooling of a polyatomic molecule. Nature 606, 70–74 (2022).

Article  CAS  PubMed  Google Scholar 

Augenbraun, B. L. et al. in Advances in Atomic, Molecular, and Optical Physics Vol. 72 (eds Dimauro, L. F. et al.) 89–182 (Elsevier, 2023).

Cheuk, L. W. et al. Λ-enhanced imaging of molecules in an optical trap. Phys. Rev. Lett. 121, 083201 (2018).

Article  CAS  PubMed  Google Scholar 

Shaw, J., Schnaubelt, J. & McCarron, D. Resonance Raman optical cycling for high-fidelity fluorescence detection of molecules. Phys. Rev. Res. 3, L042041 (2021).

Article  CAS  Google Scholar 

Schlosser, N., Reymond, G., Protsenko, I. & Grangier, P. Sub-Poissonian loading of single atoms in a microscopic dipole trap. Nature 411, 1024–1027 (2001).

Article  CAS  PubMed  Google Scholar 

Anderegg, L. et al. An optical tweezer array of ultracold molecules. Science 365, 1156–1158 (2019).

Article  CAS  PubMed  Google Scholar 

Holland, C. M., Lu, Y. & Cheuk, L. W. Bichromatic imaging of single molecules in an optical tweezer array. Phys. Rev. Lett. 131, 053202 (2023).

Article  CAS  PubMed  Google Scholar 

Vilas, N. B. et al. An optical tweezer array of ultracold polyatomic molecules. Nature https://doi.org/10.1038/s41586-024-07199-1 (2024).

Holland, C. M., Lu, Y. & Cheuk, L. W. On-demand entanglement of molecules in a reconfigurable optical tweezer array. Science 382, 1143–1147 (2023).

Article  CAS  PubMed  Google Scholar 

Bao, Y. et al. Dipolar spin-exchange and entanglement between molecules in an optical tweezer array. Science 382, 1138–1143 (2023).

Article  CAS  PubMed  Google Scholar 

Campbell, W. C. & Hudson, E. R. Dipole–phonon quantum logic with trapped polar molecular ions. Phys. Rev. Lett. 125, 120501 (2020).

Article  CAS  PubMed  Google Scholar 

Hudson, E. R. & Campbell, W. C. Laserless quantum gates for electric dipoles in thermal motion. Phys. Rev. A 104, 042605 (2021).

Article  CAS  Google Scholar 

Yu, P., Cheuk, L. W., Kozyryev, I. & Doyle, J. M. A scalable quantum computing platform using symmetric-top molecules. New J. Phys. 21, 093049 (2019).

Article  CAS  Google Scholar 

Kozyryev, I. & Hutzler, N. R. Precision measurement of time-reversal symmetry violation with laser-cooled polyatomic molecules. Phys. Rev. Lett. 119, 133002 (2017).

Article  PubMed  Google Scholar 

Guo, H. et al. Surface chemical trapping of optical cycling centers. Phys. Chem. Chem. Phys. 23, 211–218 (2021).

Article  CAS  PubMed  Google Scholar 

Wolfowicz, G. et al. Quantum guidelines for solid-state spin defects. Nat. Rev. Mater. 6, 906–925 (2021).

Article  CAS  Google Scholar 

Shuman, E. S., Barry, J. F. & DeMille, D. Laser cooling of a diatomic molecule. Nature 467, 820–823 (2010).

Article  CAS  PubMed  Google Scholar 

Hummon, M. T. et al. 2D magneto-optical trapping of diatomic molecules. Phys. Rev. Lett. 110, 143001 (2013).

Article  PubMed  Google Scholar 

Zhelyazkova, V. et al. Laser cooling and slowing of CaF molecules. Phys. Rev. A 89, 053416 (2014).

Article  Google Scholar 

Anderegg, L. et al. Radio frequency magneto-optical trapping of CaF with high density. Phys. Rev. Lett. 119, 103201 (2017).

Article  PubMed  Google Scholar 

Lim, J. et al. Laser cooled YbF molecules for measuring the electron’s electric dipole moment. Phys. Rev. Lett. 120, 123201 (2018).

Article  CAS  PubMed  Google Scholar 

Albrecht, R., Scharwaechter, M., Sixt, T., Hofer, L. & Langen, T. Buffer-gas cooling, high-resolution spectroscopy, and optical cycling of barium monofluoride molecules. Phys. Rev. A 101, 013413 (2020).

Article  CAS  Google Scholar 

Zhang, Y., Zeng, Z., Liang, Q., Bu, W. & Yan, B. Doppler cooling of buffer-gas-cooled barium monofluoride molecules. Phys. Rev. A 105, 033307 (2022).

Article  CAS  Google Scholar 

Gu, R. et al. Radiative force from optical cycling on magnesium monofluoride. Phys. Rev. A 105, 042806 (2022).

Article  CAS  Google Scholar 

Hofsäss, S. et al. Optical cycling of AlF molecules. New J. Phys. 23, 075001 (2021).

Article  Google Scholar 

Kozyryev, I. et al. Sisyphus laser cooling of a polyatomic molecule. Phys. Rev. Lett. 118, 173201 (2017).

Article  PubMed  Google Scholar 

Baum, L. et al. 1D magneto-optical trap of polyatomic molecules. Phys. Rev. Lett. 124, 133201 (2020).

Article  CAS  PubMed  Google Scholar 

Augenbraun, B. L. et al. Laser-cooled polyatomic molecules for improved electron electric dipole moment searches. New J. Phys. 22, 022003 (2020).

Article  CAS 

Comments (0)

No login
gif